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Scattering phenomena can be very complicated  even for a monochromatic light source  since the scattering is dependent on the size of the scattering sphere. In his seminal paper "Mie theory, Airy theory, and the natural rainbow" ^{1}, Raymond L. Lee used a powerful technique to illustrate how the appearance of rainbows varies with the size of the scattering water drops.
The MiePlot program can produce such "Lee diagrams", in which each coloured point represents the colour of light scattered in a specific direction by a drop of radius r  as shown in Figs. 1 and 2 (where scattering at angles between 137° and 145° has been calculated for 300 values of r between 10 µm and 1000 µm, using the "High" option for the number of wavelengths). Note that this diagram required about 30 hours of computation time!
For each value of r, the primary rainbow is depicted by a vertical column of colours. The brightness of each vertical line of colours has been normalized by the maximum luminance for that value of r.
Fig. 1 shows brightly coloured primary rainbows caused by scattering of sunlight for r between 300 µm and 1000 µm. For drops with r between 500 and 1000 µm, the brightest scattering occurs between 138° and 139°, whereas the maximum scattering for r = 10 µm drops occurs around 142°. Very small droplets of water (r < 30 µm), such as occurring those in fog or clouds, produce a rainbow that is almost white  known as fogbows or cloudbows for obvious reasons. Supernumerary arcs are not visible for r > 300 µm, but become more obvious and more widely spaced for r < 200 µm.
Fig. 1 Lee diagram for 137°  145° for uniform drops  Fig. 2 Lee diagram for 137°  145° for nonuniform drops with a standard deviation of 10% 
Comparison of Figs. 1 and 2 shows that supernumerary arcs can disappear when the water drops are nonuniform in size. For r around 100 µm, four supernumerary arcs between 141° and 145° are clearly visible for uniform drops (in Fig. 1), but they are much less visible for drops with a lognormal size distribution with a standard deviation of 10% (in Fig. 2). This effect is more obvious for larger drops, such as r > 200 µm
Fig. 3 Lee diagram for 120°  150° showing primary and secondary rainbows 
1 "Mie theory, Airy theory, and the natural rainbow", Raymond L. Lee Jr. Applied Optics, Vol. 37, No. 9, pp.15061520, 20 March 1998
N.B. This article can be downloaded free of charge (for personal use) at the above link (1.2 MB)
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